I believe wiring each of these 12-volt panels in series will leave me at 72 volts and 4.93 amps (based on reading the specs I think they're 4.93 amp panels)
NNNOOO!!! Go by the VoC number for calculating your string voltage. There's no such thing as a "12v panel", it's just a marketing term that means "Will create enough voltage to charge a 12v battery", you need to go off the VoC to get the real voltage. Call those panels 25v and divide the working PV Input by that. That'll tell you how many you can put in series.
OK, now that I've got that out of my system, let me put on my working-stiff/broke-guy hat and see about saving you a LOT of money.
Ditch/return those Gel batteries if you can. The only thing they grant you is a) not having to keep up on water levels, and b) you can hang them upside down from the ceiling if you wanted to. Go to WallyWorld and get a stack of their 29DC 122Ah Deep Cycle Marine Batteries and a jug of Distilled water. Those batteries will give you the same capacity as the Gel's (about 60Ah each at 50% DoD) but only cost about $100 each with core charge and tax. Since you'll need to buy 2 at a time to feed your 24v setup, you're still going to save about $200+ for each battery bank over the Gel's.
For those 80w panels, grab a cheapie 24v PWM controller and wire those in series to the PWM, then just connect the PWM to the battery bank and call it a day. Mixing and matching panels will take a performance hit every time, so try to keep the oddballs out of the loop. There's nothing wrong with having multiple charging systems talking to the same batteries. Since you're getting close to topping out what the MPPT controller can handle, if you put up more panels you'll do the same thing. Grab another stack of panels, another MPPT controller, and hook it up to the same batteries.
If you can swing used panels from someone like SanTan Solar or Watts247 and afford the shipping, it's a cheap way to get all the watts fast.
Yes, Victron and LiFePo4 batteries sound great, like a good juicy steak, but it sounds like your budget is Beef Top Ramen. That's OK, you can improve later when you've already got something working now. If you need to shave more money, yellow butt connectors, heat shrink, and electrical tape are all available at Harbor Freight for much cheaper than a couple dozen MC4's and the tool.
OK, it sounds like Top Ramen time for me.